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Angular Correlation and Polarization of X-rays Emitted from Highly Charged Ions

Angular Correlation and Polarization of X-rays Emitted from Highly Charged Ions
Author: Zhongwen Wu
Publisher:
Total Pages:
Release: 2017
Genre:
ISBN:

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In collisions of highly charged ions with electrons or light, ions are usually excited to one of their excited states and, then, may stabilize radiatively under the emission of fluorescence photons. Detailed studies on the emitted photons can help understand the structure and collision dynamics of the ions. When compared with total decay rates, angle-resolved properties such as angular correlation and polarization of emitted photons were found more sensitive to various interactions and effects and, actually, have helped provide new insights into electron-electron and electron-photon interactions in the presence of strong Coulomb fields. For this reason, such kind of studies has attracted considerable interest in both theory and experiment. Until now, however, almost all studies of x-ray angular correlation and polarization were performed for photons emitted from well-isolated energy levels. Little attention was paid so far to photon emissions from two or more overlapping resonances of ions. In this thesis, we develop a novel theoretical formalism to study radiative decay from the overlapping resonances. Special attention is paid to the question of how the splitting of these resonances affect the angular and polarization properties of emitted photons. Calculations are performed based on the density matrix theory and multi-configuration Dirac-Fock method. The obtained results from several case studies show that the photon angular distribution and polarization are strongly affected by the splitting and sequence of the overlapping resonances. Therefore, we suggest that accurate angle-resolved measurements of photon emissions may serve as a tool to identify level splitting and sequence of overlapping resonances in excited highly charged ions, even if they cannot be spectroscopically resolved. When applied to the isotopes with non-zero nuclear spin, moreover, such a tool can also be used to determine hyperfine splitting and associated nuclear parameters.


Nuclear Science Abstracts

Nuclear Science Abstracts
Author:
Publisher:
Total Pages: 580
Release: 1974
Genre: Nuclear energy
ISBN:

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Highly-charged Ion Collisions with Atoms

Highly-charged Ion Collisions with Atoms
Author: Renata S Cumbee
Publisher:
Total Pages: 256
Release: 2016
Genre:
ISBN:

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Atomic collisions play a fundamental role in astrophysics, plasma physics, and fusion physics. In this dissertation, we focus on charge exchange (CX) between hot ions and neutral atoms relevant to a selection of astronomical environments. Even though charge exchange calculations can provide vital information including neutral and ion density distributions, ion temperatures, elemental abundances, and ion charge state distributions in the environments considered, both theoretical calculations and laboratory studies of these processes lack the necessary reliability and/or coverage. In order to better understand the spectra we observe in astrophysical environments in which both hot plasma and neutral gas are present, including comets, the heliosphere, supernova remnants, galaxy clusters, star forming galaxies, the outflows of starburst galaxies, and cooling flows of hot gas in the intracluster medium, a thorough CX X-ray model is needed. Included in this model should be a complete set of X-ray line ratios for relevant ion and neutral interactions for a range of energies. In this work, theoretical charge exchange emission spectra are produced using cross sections calculated with widely applied approaches including the quantum mechanical molecular orbital close coupling (QMOCC), atomic orbital close coupling (AOCC), classical trajectory Monte Carlo (CTMC), and the multichannel Landau-Zener (MCLZ) methods. When possible, theoretical data are benchmarked to experiments. Using a comprehensive, but still far from complete, CX database, new models are performed for a variety of X-ray emitting environments. In an attempt to describe the excess emission in X-rays of the starburst galaxy M82, Ne X CX line ratios are compared to line ratios observed in the region. A more complete XSPEC X-ray emission model is produced for H-like and He-like C-Al ions colliding with H and He for a range of energies; 200, 300, 500, 700, 1000, 2000, 3000, and 5000 eV/u. This model is applied to the northeast rim of the Cygnus Loop supernova remnant in an attempt to determine the contribution of CX to that region. The database is also applied to a preliminary model of the fast and slow solar wind interacting with the heliosphere.


Spectroscopic Investigations of Highly Charged Ions Using X-Ray Calorimeter Spectrometers

Spectroscopic Investigations of Highly Charged Ions Using X-Ray Calorimeter Spectrometers
Author:
Publisher:
Total Pages: 164
Release: 2008
Genre:
ISBN:

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Spectroscopy of K-shell transitions in highly charged heavy ions, like hydrogen-like uranium, has the potential to yield information about quantum electrodynamics (QED) in extremely strong nuclear fields as well as tests of the standard model, specifically parity violation in atomic systems. These measurements would represent the 'holy grail' in high-Z atomic spectroscopy. However, the current state-of-the-art detection schemes used for recording the K-shell spectra from highly charged heavy ions does not yet have the resolving power to be able to attain this goal. As such, to push the field of high-Z spectroscopy forward, new detectors must be found. Recently, x-ray calorimeter spectrometers have been developed that promise to make such measurements. In an effort to make the first steps towards attaining the 'holy grail', measurements have been performed with two x-ray calorimeter spectrometers (the XRS/EBIT and the ECS) designed and built at Goddard Space Flight Center in Greenbelt, MD. The calorimeter spectrometers have been used to record the K-shell spectra of highly charged ions produced in the SuperEBIT electron beam ion trap at Lawrence Livermore National Laboratory in Livermore, CA. Measurements performed with the XRS/EBIT calorimeter array found that the theoretical description of well-above threshold electron-impact excitation cross sections for hydrogen-like iron and nickel ions are correct. Furthermore, the first high-resolution spectrum of hydrogen-like through carbon-like praseodymium ions was recorded with a calorimeter. In addition, the new high-energy array on the EBIT Calorimeter Spectrometer (ECS) was used to resolve the K-shell x-ray emission spectrum of highly charged xenon ions, where a 40 ppm measurement of the energy of the K-shell resonance transition in helium-like xenon was achieved. This is the highest precision result, ever, for an element with such high atomic number. In addition, a first-of-its-kind measurement of the effect of the generalized Breit interaction (GBI) on electron-impact excitation cross sections was performed. This measurement found that for theoretical electron-impact excitation cross sections to fit with experimental data the GBI needs to be taken into account.


Atomic and Molecular Photoabsorption

Atomic and Molecular Photoabsorption
Author: Joseph Berkowitz
Publisher: Academic Press
Total Pages: 533
Release: 2015-03-27
Genre: Science
ISBN: 0128019581

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Atomic and Molecular Photoabsorption: Partial Cross Sections is a companion work to Joseph Berkowitz's earlier work, Atomic and Molecular Photoabsorption: Absolute Total Cross Sections, published with Academic Press in 2002. In this work Joseph Berkowitz selected the "best" absolute partial cross sections for the same species as included in the companion work. A contrast, however, is that photoabsorption measurements, being of order I/Io, do not require the most intense light sources, whereas acquiring data on the products of light interactions with gaseous matter (ions, electrons, various coincidence measurements) has benefited significantly with the arrival of second- and third-generation synchrotrons. The newer devices have also extended the energy range of the light sources to include the K-shells of the species discussed here. The newer light sources encouraged experimentalists to develop improved instrumentation. Thus, the determination of partial cross sections continues to be an active field, with more recent results in some cases superseding earlier ones. Where the accuracy of the absolute partial cross sections is deemed sufficient (less than five percent), numerical tables are included in this new work. In other cases, the available data are presented graphically. Includes data on atoms, diatomic molecules, triatomic molecules, and polyatomic molecules Written by world-leading pioneer in the field of photoionization mass spectrometry Very clear presentation of the useful, quantitative information in both tables and graphs


The Polarization of Celestial X-rays

The Polarization of Celestial X-rays
Author: Joseph F. Dolan
Publisher:
Total Pages: 105
Release: 1966
Genre: Polarization (Nuclear physics)
ISBN:

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X-Ray Radiation of Highly Charged Ions

X-Ray Radiation of Highly Charged Ions
Author: Heinrich F. Beyer
Publisher: Springer Science & Business Media
Total Pages: 260
Release: 1997-08-14
Genre: Science
ISBN: 9783540631859

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This title is a comprehensive collection of atomic characteristics of highly charged ion sources and elementary processes related to X-ray radiation: energy levels, wavelengths, transition probabilities, cross sections and rate coefficients. Many figures, tables, simple formulas and scaling laws accompany the text wherever possible.