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Cavity-coupled Plasmonic Systems for Enhanced Light-matter Interactions

Cavity-coupled Plasmonic Systems for Enhanced Light-matter Interactions
Author: Abraham Vázquez-Guardado
Publisher:
Total Pages: 136
Release: 2018
Genre:
ISBN:

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Light-matter interaction is a pivotal effect that involves the synergetic interplay of electromagnetic fields with fundamental particles. In this regard localized surface plasmons (LSP) arise from coherent interaction of the electromagnetic field with the collective oscillation of free electrons in confined sub-wavelength environments. Their most attractive properties are strong field enhancements at the near field, highly inhomogeneous, peculiar temporal and spatial distributions and unique polarization properties. LSP systems also offer a unique playground for fundamental electromagnetic physics where micro-scale systemic properties can be studied in the macro-scale. These important properties and opportunities are brought up in this work where I study hybrid cavity-coupled plasmonic systems in which the weak plasmonic element is far-field coupled with the photonic cavity by properly tuning its phase. In this work I preset the fundamental understanding of such a complex systems from the multi-resonance interaction picture along experimental demonstration. Using this platform and its intricate near fields I further demonstrate a novel mechanism to generate superchiral light: a field polarization property that adds a degree of freedom to light-matter interactions at the nanoscale exploited in advanced sensing applications and surface effect processes. Finally, the detection of non-chiral analytes, such as proteins, neurotransmitters or nanoparticles, and more complex chiral analytes, such as proteins and its conformation states, amino acids or chiral molecules at low concentrations is demonstrated in several biosensing applications. The accompanied experiential demonstrations were accomplished using the nanoimprinting technique, which places the cavity-coupled hybrid plasmonic system as a unique platform towards realistic applications not limited by expensive lithographic techniques.


Plasmon-enhanced light-matter interactions

Plasmon-enhanced light-matter interactions
Author: Peng Yu
Publisher: Springer Nature
Total Pages: 348
Release: 2022-03-01
Genre: Science
ISBN: 303087544X

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This book highlights cutting-edge research in surface plasmons, discussing the different types and providing a comprehensive overview of their applications. Surface plasmons (SPs) receive special attention in nanoscience and nanotechnology due to their unique optical, electrical, magnetic, and catalytic properties when operating at the nanoscale. The excitation of SPs in metal nanostructures enables the manipulation of light beyond the diffraction limit, which can be utilized for enhancing and tailoring light-matter interactions and developing ultra-compact high-performance nanophotonic devices for various applications. With clear and understandable illustrations, tables, and descriptions, this book provides physicists, materials scientists, chemists, engineers, and their students with a fundamental understanding of surface plasmons and device applications as a basis for future developments.


Plasmonics: Fundamentals and Applications

Plasmonics: Fundamentals and Applications
Author: Stefan Alexander Maier
Publisher: Springer Science & Business Media
Total Pages: 234
Release: 2007-05-16
Genre: Technology & Engineering
ISBN: 0387378251

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Considered a major field of photonics, plasmonics offers the potential to confine and guide light below the diffraction limit and promises a new generation of highly miniaturized photonic devices. This book combines a comprehensive introduction with an extensive overview of the current state of the art. Coverage includes plasmon waveguides, cavities for field-enhancement, nonlinear processes and the emerging field of active plasmonics studying interactions of surface plasmons with active media.


Cavity Plasmonics

Cavity Plasmonics
Author: Marie-Elena Kleemann
Publisher:
Total Pages:
Release: 2019
Genre:
ISBN:

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Strong Light-matter Coupling

Strong Light-matter Coupling
Author: Leong Chuan Kwek
Publisher: World Scientific
Total Pages: 303
Release: 2013-12-23
Genre: Science
ISBN: 9814460354

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The physics of strong light-matter coupling has been addressed in different scientific communities over the last three decades. Since the early eighties, atoms coupled to optical and microwave cavities have led to pioneering demonstrations of cavity quantum electrodynamics, Gedanken experiments, and building blocks for quantum information processing, for which the Nobel Prize in Physics was awarded in 2012. In the framework of semiconducting devices, strong coupling has allowed investigations into the physics of Bose gases in solid-state environments, and the latter holds promise for exploiting light-matter interaction at the single-photon level in scalable architectures. More recently, impressive developments in the so-called superconducting circuit QED have opened another fundamental playground to revisit cavity quantum electrodynamics for practical and fundamental purposes. This book aims at developing the necessary interface between these communities, by providing future researchers with a robust conceptual, theoretical and experimental basis on strong light-matter coupling, both in the classical and in the quantum regimes. In addition, the emphasis is on new forefront research topics currently developed around the physics of strong light-matter interaction in the atomic and solid-state scenarios.


Modern Plasmonics

Modern Plasmonics
Author: Alexei A. Maradudin
Publisher: Elsevier
Total Pages: 461
Release: 2014-09-10
Genre: Science
ISBN: 0444595236

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Plasmonics is entering the curriculum of many universities, either as a stand alone subject, or as part of some course or courses. Nanotechnology institutes have been, and are being, established in universities, in which plasmonics is a significant topic of research. Modern Plasmonics offers a comprehensive presentation of the properties of surface plasmon polaritons, in systems of different structures and various natures, e.g. active, nonlinear, graded, theoretical/computational and experimental techniques for studying them, and their use in a variety of applications. Contains material not found in existing books on plasmonics, including basic properties of these surface waves, theoretical/computational and experimental approaches, and new applications of them Each chapter is written by an expert in the subject to which it is devoted Emphasis on applications of plasmonics that have been realized, not just predicted or proposed


Exploring Plasmonic-photonic Coupled Systems Using Microcavity-based Single-particle Spectroscopy

Exploring Plasmonic-photonic Coupled Systems Using Microcavity-based Single-particle Spectroscopy
Author: FENG PAN
Publisher:
Total Pages: 0
Release: 2022
Genre:
ISBN:

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Control of light-matter interactions is important for a variety of applications, such as sensing, photocatalysis, and information science, to name a few. Recently, plasmonic-photonic coupled systems, which inherit ultrahigh-quality factor and ultrasmall mode volume from their component cavities, have shown promise in tailoring light-matter interactions. Understanding energy dynamics in such coupled systems which dictate multiple dissipation pathways and couplings, sheds light upon the rational design of optimal coupled systems, for instance, achieving disparity between couplings and dissipations for strong coupling and precisely controlling photon transfer rates between component cavities in photonic circuits. The core of my thesis examines a model system, i.e., a whispering-gallery-mode (WGM) microcavity coupled to a gold nanorod that supports localized surface plasmon (LSP), and addresses two main questions, i.e., how to elucidate system parameters and how to control them. I will present a new way that combines simultaneous measurement of absorption and transmission with theoretical modeling, to pin down eight system parameters spanning up to 9 orders of magnitude. I then demonstrate a solvent-embedding strategy to actively control plasmonic-photonic interactions in a microbubble cavity. Chloroform that has similar refractive index to the material of the microbubble cavity, is chosen to fill the microbubble for increasing the mode overlap between LSP and WGMs. The effect of modulating interior dielectric environment on mode volume and mode overlap is thoroughly interrogated through both experiments and optical simulations. In addition, I will demonstrate two most recent applications under the theme of plasmonics and photonics, i.e., single-particle photothermal imaging through high-Q all-glass WGM microcavities and plasmonic enhancement for electrocatalysis, respectively.


Plasmonic Control of Light Emission

Plasmonic Control of Light Emission
Author: Young Chul Jun
Publisher: Stanford University
Total Pages: 138
Release: 2010
Genre:
ISBN:

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Enhanced light-matter interactions in light-confining structures (such as optical cavities) have been extensively investigated for both fundamental studies and practical applications. Plasmonic nanostructures, which can confine and manipulate light down to ~1 nm scale, are becoming increasingly important. Many areas of optical physics and devices can benefit from such extreme light concentration and manipulation. For example, fluorescent molecule or quantum dot (QD) emission can be strongly modified and controlled via surface plasmon polariton (SPP) coupling. In this dissertation, we present our theoretical and experimental studies on QD emission in metal nanogap structures that can provide extreme field concentration, enhancing light-matter interactions significantly. We start with a theoretical analysis of dipole emission in metal-dielectric-metal (MDM) waveguide structures. We look at both infinite (i.e. planar) and finite thickness MDM structures. We find that both structures exhibit strong spontaneous emission enhancements due to the tight confinement of modes between two metallic plates and that light emission is dominated by gap SPP coupling. For planar structures we present analytical solutions for the enhanced dipole decay rate, while for finite thickness MDM structures (i.e. nanoslits) we present results from numerical simulations. Next, we present our experiments on the SPP coupling of CdSe/ZnS QD emission in metal nanoslits. First, we observed clear lifetime and polarization state changes of QD emission with slit width due to gap SPP excitation. Second, with optimized side grooves (i.e. combined slit-groove and hole-groove structures), we collimated QD emission vertically into a very narrow angle, achieving an unprecedented level of directionality control, and visualized it with confocal scanning microscopy. Third, by using two metal plates as electrodes, we dynamically modulated the QD emission intensity and wavelength with external voltage. Finally, we extend our dipole emission calculation to several slot waveguide structures. We consider light emission in metal slots, metal-oxide-Si slots, and Si slot waveguides. We find that large spontaneous emission enhancements can be obtained over a broad range of wavelengths and that light emission is strongly funneled into slot waveguide modes. These represent broadband waveguide QED (quantum electro-dynamics) systems, which have unique merits for on-chip light sources and quantum information processing. These theoretical and experimental studies show that the SPP coupling of light emission is a very promising way to control light emission properties and may find broad application in spectroscopy, sensing, optoelectronics, and integrated optics.


Light-Matter Interactions Towards the Nanoscale

Light-Matter Interactions Towards the Nanoscale
Author: Maura Cesaria
Publisher: Springer Nature
Total Pages: 348
Release: 2022-05-14
Genre: Science
ISBN: 9402421386

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The investigation of light-matter interactions in materials, especially those on the nanoscale, represents perhaps the most promising avenue for scientific progress in the fields of photonics and plasmonics. This book examines a variety of topics, starting from fundamental principles, leading to the current state of the art research. For example, this volume includes a chapter on the sensing of biological molecules with optical resonators (microspheres) combined with plasmonic systems, where the response this system are described in a fundamental and elegant manner using coupled mode theory. Symmetry plays a major role in the book. One chapter on time reversal symmetry in electromagnetic theory describes how to control the properties of light (e.g. scattering and directionality of the flow of light) in materials with certain topological invariants. Another chapter where symmetry is prominent reformulates, using a gentle and pedagogical approach, Maxwell’s Equations into a new set of fields that reveal a “handedness” symmetry in electromagnetic theory, which can be applied to photonic systems in, for example, the sensing of chiral molecules and understanding the conditions for zero reflection. Also, for students and researchers starting in the field of nanoplasmonics, the book includes a tutorial on the finite element time domain simulation of nanoplasmonic systems. Other topics include photonic systems for quantum computing, nanoplasmonics, and optical properties of nano and bulk materials. The authors take a pedagogical approach to their topic, making the book an excellent reference for graduate students and scientists starting in the fields of photonics or plasmonics.


Quantum Plasmonics

Quantum Plasmonics
Author: Sergey I. Bozhevolnyi
Publisher: Springer
Total Pages: 338
Release: 2016-11-26
Genre: Science
ISBN: 3319458205

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This book presents the latest results of quantum properties of light in the nanostructured environment supporting surface plasmons, including waveguide quantum electrodynamics, quantum emitters, strong-coupling phenomena and lasing in plasmonic structures. Different approaches are described for controlling the emission and propagation of light with extreme light confinement and field enhancement provided by surface plasmons. Recent progress is reviewed in both experimental and theoretical investigations within quantum plasmonics, elucidating the fundamental physical phenomena involved and discussing the realization of quantum-controlled devices, including single-photon sources, transistors and ultra-compact circuitry at the nanoscale.